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US4332909A Expired / Lapsed US ⏱️ 0.0 years remaining

Silicon nitride based sintered product and method of producing the same

Assignee: Toshiba Corp
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Filing: 1980-08-25
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Granted: 1982-06-01
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Expires: 2000-08-25
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Abstract

Abstract A silicon nitride based sintered product produced by sintering a powder mixture consisting essentially of silicon nitride, at least one oxide of yttrium, scandium, cerium, lanthanum and the metals of lanthanide series and at least one metal or metal oxide of iron, nickel and cobalt.

Inventors

  • 👤 Katsutoshi Nishida
  • 👤 Toshihiko Ochiai

Bibliographic Details

Application Number —
Jurisdiction US
Data Source google_patents
Last Synchronized 2026-10-30 10:35
CPC Classifications
C; C04; C04B; C04B35/00; C04B35/515; C04B35/58; C04B35/584; C04B35/593; C04B35/597

Claims Analysis

Total Claims: 26
Claim 1
Independent Claim 60 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt.
Claim 2
Dependent Claim 60 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt.
Claim 3
Dependent Claim 28 words
The composition of claim 1, wherein the oxides of yttrium, scandium, cerium, lanthanum and the metals of lanthanide series are present in from 1 to 5 weight parts.
Claim 4
Dependent Claim 25 words
The composition of claim 1 or 2, wherein the metal oxide of iron, nickel and cobalt is present in from 2 to 50 volume parts.
Claim 5
Dependent Claim 96 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the metal oxide of iron, nickel and cobalt is replaced by at least one metal or metal oxide of molybdenum, tungsten, chromium and manganese, in the amount of up to 20 percent by weight.
Claim 6
Dependent Claim 96 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the metal oxide of iron, nickel and cobalt is replaced by at least one metal or metal oxide of molybdenum, tungsten, chromium and manganese, in the amount of up to 20 percent by weight.
Claim 7
Dependent Claim 82 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the silicon nitride is replaced by chemcially stable refractory compound, in the amount of less than 50 percent by volume.
Claim 8
Dependent Claim 82 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the silicon nitride is replaced by chemcially stable refractory compound, in the amount of less than 50 percent by volume.
Claim 9
Dependent Claim 35 words
The composition of claim 5, wherein the chemically stable refractory compound is at least one of aluminum nitride, titanium nitride, zirconium nitride, titanium carbide, zirconium carbide, silicon carbide, chromium silicide, tungsten silicide and molybdenum silicide.
Claim 10
Dependent Claim 80 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt; and a sintering aid in the amount of less than 10 weight parts per 100 weight parts of silicon nitride.
Claim 11
Dependent Claim 80 words
A composition consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt; and a sintering aid in the amount of less than 10 weight parts per 100 weight parts of silicon nitride.
Claim 12
Dependent Claim 27 words
The composition of claim 7, wherein the sintering aid is at least one of aluminum oxide, magnesium oxide, silica, boron oxide, lithium oxide and the oxide spinels.
Claim 13
Dependent Claim 69 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt.
Claim 14
Dependent Claim 69 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt.
Claim 15
Dependent Claim 29 words
The sintered product of claim 1, wherein the oxides of yttrium, scandium, cerium, lanthanum and the metals of lanthanide series are present in from 1 to 5 weight parts.
Claim 16
Dependent Claim 26 words
The sintered product of claim 9 or 10, wherein the metal oxide of iron, nickel and cobalt is present in from 2 to 50 volume parts.
Claim 17
Dependent Claim 105 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the metal oxide of iron, nickel and cobalt is replaced by at least one metal or metal oxide of molybdenum, tungsten, chromium and manganese, in the amount of up to 20 percent by weight.
Claim 18
Dependent Claim 105 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the metal oxide of iron, nickel and cobalt is replaced by at least one metal or metal oxide of molybdenum, tungsten, chromium and manganese, in the amount of up to 20 percent by weight.
Claim 19
Dependent Claim 91 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the silicon nitride is replaced by chemically stable refractory compound, in the amount of less than 50 percent by volume.
Claim 20
Dependent Claim 91 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; and 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt, wherein the silicon nitride is replaced by chemically stable refractory compound, in the amount of less than 50 percent by volume.
Claim 21
Dependent Claim 36 words
The sintered product of claim 13, wherein the chemically stable refractory compound is at least one of aluminum nitride, titanium nitride, zirconium nitride, titanium carbide, zirconium carbide, silicon carbide, chromium silicide, tungsten silicide and molybdenum silicide.
Claim 22
Dependent Claim 89 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt; and a sintering aid in the amount of less than 10 weight parts per 100 weight parts of silicon nitride.
Claim 23
Dependent Claim 89 words
A sintered product which is produced by sintering a powder mixture consisting essentially of silicon nitride, 0.02 to 10 weight parts per 100 weight parts of silicon nitride of at least one oxide of yttrium, scandium, cerium, lanthanum and the metal oxides of the lanthanide series; 1 to 100 volume parts per 100 volume parts of silicon nitride of at least one metal oxide of iron, nickel and cobalt; and a sintering aid in the amount of less than 10 weight parts per 100 weight parts of silicon nitride.
Claim 24
Dependent Claim 28 words
The sintered product of claim 15, wherein the sintering aid is at least one of aluminum oxide, magnesium oxide, silica, boron oxide, lithium oxide and the oxide spinels.
Claim 25
Dependent Claim 17 words
The sintered product of claim 9, wherein the sintering temperature is from 1400° C. to 1900° C.
Claim 26
Dependent Claim 17 words
The sintered product of claim 9, wherein the sintering temperature is from 1500° C. to 1800° C.

References Cited (Backward Citations)

US3409417A Cited
US3969125A Cited
US3830652A Cited
US4143107A Cited
US4073845A Cited
US4102698A Cited
JPS5499114A Cited

USPTO Annuity & Maintenance Windows

Annuity Stage Window Opens Payment Deadline Surcharge Period Until Estimated Fee Status
3.5 Years (Year 4) 1985-05-31 1985-11-30 1986-06-01 $2000.00 Window Closed / Lapsed
7.5 Years (Year 8) 1989-05-31 1989-11-30 1990-06-01 $3760.00 Window Closed / Lapsed
11.5 Years (Year 12) 1993-05-31 1993-11-30 1994-06-01 $7700.00 Window Closed / Lapsed

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