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US3882015A Expired / Lapsed US ⏱️ 0.0 years remaining

Countercurrent catalytic contact of a reactant stream in a multi-stage process and the apparatus therefor

Assignee: Universal Oil Products Co
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Filing: 1973-05-29
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Granted: 1975-05-06
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Expires: 1993-05-29
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Abstract

Abstract A unitary, multiple-stage reaction system for countercurrently contacting a fluid reactant stream with catalyst particles which are movable through said system via gravity-flow. Especially adaptable for use in both endothermic and exothermic conversion systems, the present reaction chamber provides for the introduction of a heat-exchange fluid between stages.

Inventors

  • 👤 Don B Carson

Bibliographic Details

Application Number —
Jurisdiction US
Data Source google_patents
Last Synchronized 2026-11-08 20:05
CPC Classifications
B; B01; B01J; B01J8/00; B01J8/08; B01J8/12; B01J8/125; B01J8/0015; B01J8/003; B01J8/02; B01J8/04; B01J8/0403; B01J8/0407; B01J8/0415; C; C10; C10G; C10G2400/00; C10G2400/26

Claims Analysis

Total Claims: 11
Claim 1
Independent Claim 349 words
A unitary, multiple-stage reaction system for countercurrently contacting a fluid reactant stream with catalyst particles movable through said system via gravity-flow, which system comprises, in combination: a. a tubular-form, vertically-disposed reaction chamber; b. at least two reaction zones withiN said chamber, each of said zones having coaxially-disposed inner and outer tubular form, catalyst-retaining screens forming (i) an annular-form catalyst holding section therebetween, (ii) an annular-form void volume between the outer screen and the interior wall of said chamber and, (iii) a center reactant conduit, said reaction zones spaced apart to form a mixing zone therebetween; c. a lower, imperforate transverse partition connected to said inner and outer screens, and to the interior wall of said chamber, said lower partition terminating at said inner catalyst-retaining screen, whereby at least one of said center reactant conduits is in open communication, at its lower extremity, with a mixing zone; d. an upper, imperforate transverse partition, across said reactant conduit, connected to said inner and outer catalyst-retaining screens, said upper partition terminating at said outer screen, whereby at least one of said annular-form void volumes is in open communication, at its upper extremity, with said mixing zone; e. catalyst-transfer conduits connecting a catalyst-holding section with the next succeeding lower catalyst-holding section, and catalyst-withdrawal conduits in the lowermost of said catalyst-holding sections, said withdrawal conduits extending downwardly through the lower extremity of said chamber, whereby catalyst particles flow via gravity from one catalyst-holding section to a lower catalyst-holding section and out of said reaction chamber; f. a reactant stream inlet port in the bottom of said reaction chamber, in open communication with the lowermost center reactant conduit; g. a catalyst inlet port in the upper end of said chamber, in open communication, via catalyst-transfer conduits, with the uppermost catalyst-holding section; h. a reaction product outlet port in the upper end of said chamber, in open communication with the uppermost annular-form void volume; and, i. a heat exchange fluid inlet conduit between said reaction zones, said inlet conduit terminating within the mixing zone therebetween and being positioned to discharge upwardly into said center reactant conduit.
Claim 2
Dependent Claim 349 words
A unitary, multiple-stage reaction system for countercurrently contacting a fluid reactant stream with catalyst particles movable through said system via gravity-flow, which system comprises, in combination: a. a tubular-form, vertically-disposed reaction chamber; b. at least two reaction zones withiN said chamber, each of said zones having coaxially-disposed inner and outer tubular form, catalyst-retaining screens forming (i) an annular-form catalyst holding section therebetween, (ii) an annular-form void volume between the outer screen and the interior wall of said chamber and, (iii) a center reactant conduit, said reaction zones spaced apart to form a mixing zone therebetween; c. a lower, imperforate transverse partition connected to said inner and outer screens, and to the interior wall of said chamber, said lower partition terminating at said inner catalyst-retaining screen, whereby at least one of said center reactant conduits is in open communication, at its lower extremity, with a mixing zone; d. an upper, imperforate transverse partition, across said reactant conduit, connected to said inner and outer catalyst-retaining screens, said upper partition terminating at said outer screen, whereby at least one of said annular-form void volumes is in open communication, at its upper extremity, with said mixing zone; e. catalyst-transfer conduits connecting a catalyst-holding section with the next succeeding lower catalyst-holding section, and catalyst-withdrawal conduits in the lowermost of said catalyst-holding sections, said withdrawal conduits extending downwardly through the lower extremity of said chamber, whereby catalyst particles flow via gravity from one catalyst-holding section to a lower catalyst-holding section and out of said reaction chamber; f. a reactant stream inlet port in the bottom of said reaction chamber, in open communication with the lowermost center reactant conduit; g. a catalyst inlet port in the upper end of said chamber, in open communication, via catalyst-transfer conduits, with the uppermost catalyst-holding section; h. a reaction product outlet port in the upper end of said chamber, in open communication with the uppermost annular-form void volume; and, i. a heat exchange fluid inlet conduit between said reaction zones, said inlet conduit terminating within the mixing zone therebetween and being positioned to discharge upwardly into said center reactant conduit.
Claim 3
Dependent Claim 38 words
The reaction system of claim 1 further characterized in that said chamber contains three reaction zones and a second heat exchange fluid inlet conduit is positioned to terminate the discharge upwardly into the second of said reaction zones.
Claim 4
Dependent Claim 226 words
A PROCESS FOR EFFECTING THE MULTIPLE-STAGE, COUNTERCURRENT CONTACT AND CONVERSION OF A REACTANT STREAM WITH CATALYST PARTICALES MOVABLE THROUGH SAID STAGES VIA GRAVITY-FLOW, WHICH PROCESS COMPRISES THE STEPS OF: A. INTRODUCING SAID REACTANT STREAM INTO A CENTRAL, LOWER PORTION OF AN ELONGATED REACTION CHAMBER CONTAINING SAID MULTIPLE STAGES; B. PASSING SAID REACTANT STREAM LATERALLY, IN RADIAL FLOW, THROUGH A FIRST ANNULAR-FORM CATALYST BED IN WHICH THE CATALYST PARTICLES ARE MOVABLE VIA GRAVITY-FLOW, AND INTO A MIXING ZONE ABOVE SAID FIRST CATALYST BED; C. INTRODUCING A HEAT-EXCHANGE FLUID INTO SAID MIXING ZONE AND PASSING THE SAME UPWARDLY, IN ADMIXTURE WITH THE REACTANT STREAM EFFLUENT, INTO THE LOWER PORTION OF A CENTER REACTANT STREAM CONDUIT, AND FLOWING SAID MIXTURE LATERALLY THROUGH A SECOND ANNULAR-FORM CATALYST BED IN WHICH THE CATALYST PARTICLES ARE MOVABLE VIA GRAVITY-FLOW; AND, D. WITHDRAWING THE RESULTING CONVERTED REACTANT STREAM FROM AN UPPER PORTION OF SAID SECOND ANNULAR-FORM CATALYST BED. F. ALLOWING SAID FILLER PARTICLES IN THE SECOND PORTION OF SAID MIXTURE TO SETTLE UPON AND WITHOUT DISPLACING SAID FIRSTPLACED STRATUM TO FORM UPPER AND LOWER LAYERS AS IN STEP (C), G. PLACING ON SAID SECOND PORTION UPPER LAYER A SECOND REINFORCING STRATUM OF SAID GLASS FIBER WHICH SINKS AND RESTS UPON SAID SECOND PORTION LOWER LAYER OF FILLER PARTICLES, AND H. CURING ALL PORTIONS OF SAID POLYESTER RESIN TO PRODUCE A UNIFIED COMPONENT THEREOF.
Claim 5
Dependent Claim 226 words
A PROCESS FOR EFFECTING THE MULTIPLE-STAGE, COUNTERCURRENT CONTACT AND CONVERSION OF A REACTANT STREAM WITH CATALYST PARTICALES MOVABLE THROUGH SAID STAGES VIA GRAVITY-FLOW, WHICH PROCESS COMPRISES THE STEPS OF: A. INTRODUCING SAID REACTANT STREAM INTO A CENTRAL, LOWER PORTION OF AN ELONGATED REACTION CHAMBER CONTAINING SAID MULTIPLE STAGES; B. PASSING SAID REACTANT STREAM LATERALLY, IN RADIAL FLOW, THROUGH A FIRST ANNULAR-FORM CATALYST BED IN WHICH THE CATALYST PARTICLES ARE MOVABLE VIA GRAVITY-FLOW, AND INTO A MIXING ZONE ABOVE SAID FIRST CATALYST BED; C. INTRODUCING A HEAT-EXCHANGE FLUID INTO SAID MIXING ZONE AND PASSING THE SAME UPWARDLY, IN ADMIXTURE WITH THE REACTANT STREAM EFFLUENT, INTO THE LOWER PORTION OF A CENTER REACTANT STREAM CONDUIT, AND FLOWING SAID MIXTURE LATERALLY THROUGH A SECOND ANNULAR-FORM CATALYST BED IN WHICH THE CATALYST PARTICLES ARE MOVABLE VIA GRAVITY-FLOW; AND, D. WITHDRAWING THE RESULTING CONVERTED REACTANT STREAM FROM AN UPPER PORTION OF SAID SECOND ANNULAR-FORM CATALYST BED. F. ALLOWING SAID FILLER PARTICLES IN THE SECOND PORTION OF SAID MIXTURE TO SETTLE UPON AND WITHOUT DISPLACING SAID FIRSTPLACED STRATUM TO FORM UPPER AND LOWER LAYERS AS IN STEP (C), G. PLACING ON SAID SECOND PORTION UPPER LAYER A SECOND REINFORCING STRATUM OF SAID GLASS FIBER WHICH SINKS AND RESTS UPON SAID SECOND PORTION LOWER LAYER OF FILLER PARTICLES, AND H. CURING ALL PORTIONS OF SAID POLYESTER RESIN TO PRODUCE A UNIFIED COMPONENT THEREOF.
Claim 6
Dependent Claim 33 words
The process of claim 3 further characterized in that said reaction chamber contains three annular-form movable catalyst beds and a heat-exchange fluid medium is introduced into each of the two mixing zones therebetween.
Claim 7
Dependent Claim 23 words
The process of claim 3 further characterized in that said heat-exchange fluid effects an increase in the temperature of said reactant stream effluent.
Claim 8
Dependent Claim 23 words
The process of claim 3 further characterized in that said heat-exchange fluid effects a decrease in the temperature of said reactant stream effluent.
Claim 9
Dependent Claim 15 words
The process of claim 3 further characterized in that said heat-exchange fluid comprises a hydrocarbon.
Claim 10
Dependent Claim 14 words
The process of claim 3 further characterized in that said heat-exchange fluid comprises hydrogen.
Claim 11
Dependent Claim 14 words
The process of claim 3 further characterized in that said heat-exchange fluid comprises steam.

References Cited (Backward Citations)

US2922757A Cited
US3647680A Cited
US3706536A Cited

USPTO Annuity & Maintenance Windows

Annuity Stage Window Opens Payment Deadline Surcharge Period Until Estimated Fee Status
3.5 Years (Year 4) 1978-05-05 1978-11-04 1979-05-06 $2000.00 Window Closed / Lapsed
7.5 Years (Year 8) 1982-05-05 1982-11-04 1983-05-06 $3760.00 Window Closed / Lapsed
11.5 Years (Year 12) 1986-05-05 1986-11-04 1987-05-06 $7700.00 Window Closed / Lapsed

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