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US4174954A Expired / Lapsed US ⏱️ 0.0 years remaining

Method for converting a reaction mixture consisting of hydrocarbon-containing fuel and an oxygen-containing gas into a fuel gas

Assignee: Siemens AG
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Filing: 1978-02-17
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Granted: 1979-11-20
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Expires: 1998-02-17
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Abstract

Abstract In a gas generation method in which liquid fuel is catalytically reacted with air at elevated temperatures to form a fuel gas, several plates each having a multiplicity of passage openings are arranged in tandem in spaced fashion within the reaction chamber of the gas generator and are embedded in a bed of packing material with the thermal conductivity of the plates higher than that of the packing material in order to obtain more uniform heating of the reaction chamber and better mixing and distribution of the reacting media permitting the gas generator to be loaded more heavily.

Inventors

  • 👤 Walter Kusebauch
  • 👤 Hana Kostka
  • 👤 Hans-Joachim Henkel
  • 👤 Christian Koch
  • 👤 Eugen S. de Bucs
  • 👤 Theo Weber

Bibliographic Details

Application Number —
Jurisdiction US
Data Source google_patents
Last Synchronized 2026-11-04 00:34
CPC Classifications
F; F02; F02M; F02M27/00; F02M27/02; B; B01; B01J; B01J8/00; B01J8/02; B01J8/0292; B01J8/04; B01J8/0446; B01J8/0449; B01J8/0453; C; C01; C01B; C01B3/00; C01B3/02; C01B3/32; C01B3/34; C01B3/38; C01B3/386; B01J2208/00; B01J2208/00008; B01J2208/00017; B01J2208/00513; B01J2208/00796; B01J2208/00884; B01J2208/00938; C01B2203/00; C01B2203/02; C01B2203/025; C01B2203/0261; C01B2203/08; C01B2203/0805; C01B2203/0838; C01B2203/0844; C01B2203/0872; C01B2203/0883; C01B2203/10; C01B2203/1005; C01B2203/1011; C01B2203/1041; C01B2203/1047; C01B2203/1052; C01B2203/1082; C01B2203/12; C01B2203/1205; C01B2203/1211; C01B2203/1235; C01B2203/1247; C01B2203/1276; C01B2203/1288; C01B2203/1294; C01B2203/16; C01B2203/1614; C01B2203/1619

Claims Analysis

Total Claims: 21
Claim 1
Independent Claim 135 words
A method of converting a reaction mixture consisting of atomized, vaporized or evaporated liquid, hydrocarbon fuel and a gas containing oxygen into a fuel gas at an elevated temperature in a gas generator including a reaction chamber comprising (a) imbedding a plurality of plates comprising porous ceramic sintered slabs containing a multiplicity of passage openings and having a surface which is catalytically active with respect to hydrocarbon fuels in a bed of packing material made up of a plurality of packing material grains such that said plates are diposed spaced one behind the other perpendicular to the flow direction of the reactants through the reaction chamber, said plates having a higher thermal conductivity than the packing material bed; and (b) passing the reaction mixture through said reaction chamber to convert it into a fuel gas.
Claim 2
Independent Claim 135 words
A method of converting a reaction mixture consisting of atomized, vaporized or evaporated liquid, hydrocarbon fuel and a gas containing oxygen into a fuel gas at an elevated temperature in a gas generator including a reaction chamber comprising (a) imbedding a plurality of plates comprising porous ceramic sintered slabs containing a multiplicity of passage openings and having a surface which is catalytically active with respect to hydrocarbon fuels in a bed of packing material made up of a plurality of packing material grains such that said plates are diposed spaced one behind the other perpendicular to the flow direction of the reactants through the reaction chamber, said plates having a higher thermal conductivity than the packing material bed; and (b) passing the reaction mixture through said reaction chamber to convert it into a fuel gas.
Claim 3
Dependent Claim 21 words
The method according to claim 1 wherein the largest dimension of the packing material grains is about 1 to 6 mm.
Claim 4
Dependent Claim 21 words
The improvement according to claim 2 wherein the smallest dimension of said packing material grains is at least about 0.8 mm.
Claim 5
Dependent Claim 18 words
The method according to claim 1 wherein the spacing of said plates is about 5 to 20 mm.
Claim 6
Dependent Claim 22 words
The method according to claim 1 wherein said packing material has a surface which is catalytically active with respect to hydrocarbon fuels.
Claim 7
Dependent Claim 18 words
The method according to claim 1 wherein said sintered slabs have a thickness of 5 to 20 mm.
Claim 8
Dependent Claim 23 words
The method according to claim 6 wherein said sintered slabs have about 10 to 100 passage openings per cm 2 of plate area.
Claim 9
Dependent Claim 19 words
The method according to claim 7 wherein the diameter of said passage openings is between 0.6 and 3 mm.
Claim 10
Dependent Claim 34 words
The method according to claim 8 wherein said sintered slabs have a thickness of about 10 mm and about 40 pasage openings of about 1 mm diameter for each cm 2 of plate area.
Claim 11
Dependent Claim 20 words
The method according to claim 6 wherein the porosity of said sintered slabs is about 20 to 60% by volume.
Claim 12
Dependent Claim 21 words
The method according to claim 6 wherein the open porosity of said sintered slabs is about 100 to 250% by volume.
Claim 13
Independent Claim 132 words
A method of converting a reaction mixture consisting of atomized, vaporized or evaporated liquid, hydrocarbon fuel and a gas containing oxygen into a fuel gas at an elevated temperature in a gas generator including a reaction chamber comprising (a) packing a plurality of plates made of a metallic material and containing a multiplicity of passage openings within the reaction chamber in a bed of plurality of packing material grains of a material which is catalytically active with respect to hydrocarbon fluids, such that said plates are disposed spaced one behind the other perpendicular to the flow direction of the reactants through the reaction chamber, said plates having higher thermal conductivity than said packing material bed; and (b) passing the reaction mixture through said reaction chamber to convert it into a fuel gas.
Claim 14
Independent Claim 132 words
A method of converting a reaction mixture consisting of atomized, vaporized or evaporated liquid, hydrocarbon fuel and a gas containing oxygen into a fuel gas at an elevated temperature in a gas generator including a reaction chamber comprising (a) packing a plurality of plates made of a metallic material and containing a multiplicity of passage openings within the reaction chamber in a bed of plurality of packing material grains of a material which is catalytically active with respect to hydrocarbon fluids, such that said plates are disposed spaced one behind the other perpendicular to the flow direction of the reactants through the reaction chamber, said plates having higher thermal conductivity than said packing material bed; and (b) passing the reaction mixture through said reaction chamber to convert it into a fuel gas.
Claim 15
Dependent Claim 33 words
The method according to claim 12 wherein the total of the cross section area per unit area of the metal plates of the passage openings increases toward the edges of the metal plates.
Claim 16
Independent Claim 135 words
A method of converting a reaction mixture consisting of atomized, vaporized or evaporated liquid, hydrocarbon fuel and a gas containing oxygen into a fuel gas at an elevated temperature in a gas generator including a reaction chamber comprising (a) packing a plurality of plates made of molybdenum silicide each of said plates having a multiplicity of passage openings in a packing material bed of a plurality of packing material grains of a material which is catalytically active with respect to hydrocarbon fuels, such that said plates are arranged spaced one behind the other perpendicular to the flow direction of the reactants through the reaction chamber, said molybdenum silicide having a higher thermal conductivity than said packing material bed; and (b) passing the reaction mixture through said reaction chamber to convert it into a fuel gas.
Claim 17
Independent Claim 135 words
A method of converting a reaction mixture consisting of atomized, vaporized or evaporated liquid, hydrocarbon fuel and a gas containing oxygen into a fuel gas at an elevated temperature in a gas generator including a reaction chamber comprising (a) packing a plurality of plates made of molybdenum silicide each of said plates having a multiplicity of passage openings in a packing material bed of a plurality of packing material grains of a material which is catalytically active with respect to hydrocarbon fuels, such that said plates are arranged spaced one behind the other perpendicular to the flow direction of the reactants through the reaction chamber, said molybdenum silicide having a higher thermal conductivity than said packing material bed; and (b) passing the reaction mixture through said reaction chamber to convert it into a fuel gas.
Claim 18
Dependent Claim 15 words
The method according to claim 14 wherein said molybdenum silicide plates carry catalytically active components
Claim 19
Dependent Claim 18 words
The method according to claim 14 and further including a gas-tight silicon dioxide coating on said molybdenum silicide.
Claim 20
Dependent Claim 29 words
The method according to claim 14 and further including disposing bodies of metallic material with wall surfaces extending parallel to the flow direction arranged in the packing material bed.
Claim 21
Dependent Claim 19 words
The method according to claim 17 wherein said bodies consist of molybdenum silicide with a gas-tight silicon dioxide coating.

References Cited (Backward Citations)

US1030508A Cited
DE482157C Cited
US2127561A Cited
US3362787A Cited
US3595626A Cited
US3828736A Cited
US3754870A Cited
US4026248A Cited

USPTO Annuity & Maintenance Windows

Annuity Stage Window Opens Payment Deadline Surcharge Period Until Estimated Fee Status
3.5 Years (Year 4) 1982-11-19 1983-05-21 1983-11-20 $2000.00 Window Closed / Lapsed
7.5 Years (Year 8) 1986-11-19 1987-05-21 1987-11-20 $3760.00 Window Closed / Lapsed
11.5 Years (Year 12) 1990-11-19 1991-05-21 1991-11-20 $7700.00 Window Closed / Lapsed

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